题目:

Robust perovskite lattice for durable and efficient pure-red light-emitting diodes


作者:

Xin Zhou1, Zhenwei Ren1,*, Jing Wang2, Zhiyong Zheng1, Hua Chen1, Bin Hu1, Chengzhao Luo1, Yu Chen1,3,*


单位:

1 School of Optoelectronic Science and Engineering & Collaborative Innovation Center of Suzhou Nano Science and Technology, Soochow University, Suzhou 215006, China

2 School of Physical Science and Technology, Ningbo University, Ningbo 315211, China

3 National University of Singapore Suzhou Research Institute, Dushu Lake Science and Education Innovation District, Suzhou 215123, China


摘要:

金属卤化物钙钛矿发光二极管在下一代显示技术中极具竞争力。然而,钙钛矿晶格结构的“柔软”特性使其光学性质对外部环境高度敏感,限制了器件的电致发光稳定性和效率。为此,陈煜、任振伟等人提出了稳固钙钛矿晶格的新方法,揭示了刚性环状铵离子与静电相互作用协同增强晶格稳固性机制,获得了高结构刚性、高稳定性的纯红光发光材料。该方法提高了材料体积模量、降低了键角波动幅度,抑制了传统软晶格钙钛矿的电场诱导畸变与离子迁移现象,促进了载流子的辐射复合。最终,器件在638 nm纯红光波段下,实现了31.3%的峰值效率与343.3小时的工作寿命。同时,验证了该方法在提升蓝光和绿光器件性能的兼容性,获得了峰值效率24.2%与27.1%的蓝光(488 nm)和绿光(523 nm)器件。该研究成果为设计、制备稳定高效钙钛矿发光器件提供了坚实的实验与理论依据。


影响因子:18.1

分区情况:一区

链接:https://www.nature.com/articles/s41467-026-79295-x